Emulsion solvents (ES), that are liquid absorbent-based CO2 seize supplies, are developed as easy and expandable droplets to regulate CO2 seize efficiency. An aqueous NaOH resolution, which is a chemical absorbent, is encapsulated by functionalized carbon nanotubes (CNTs) to kind a strong adsorbent by enhancing the excessive lipophilicity and high-viscosity silicone oil. The ratio of every part controls the CO2 seize efficiency of the solvent. It’s proven that droplets of NaOH aqueous resolution shaped in fantastic sizes enhance the effectivity of the chemical response capability of NaOH and CO2, and thus, even when crystallization happens, they can be utilized in a stationary atmosphere, and NaOH can be utilized at a excessive focus. It’s discovered that the optimum focus of CNTs required to reduce the dimensions of the emulsion is 0.075 wt%, whereas the CO2 seize capability is 2.23 mmolCO2 g−1ES–NaOH at a pure CO2 focus and 1.31 mmolCO2 g−1ES–NaOH at a low CO2 focus (2000 ppm, 50% relative humidity). The oil part may be recycled constantly by separating the crystallized aqueous part after the CO2 seize. These outcomes exhibit that chemical absorbents with wonderful CO2 seize efficiency can be utilized safely and for a very long time to be able to scale back indoor CO2, and the CO2 seize efficiency may be flexibly managed.